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Aalborg Universitet Particulate emissions from residential wood combustion Improving estimations in Denmark and Portugal Luis Teles de Carvalho, Ricardo; Jensen, Ole Michael; Tarelho, Luis A. C.; Olesen, Helge Rørdam

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Aalborg Universitet

Particulate emissions from residential wood combustion Improving estimations in Denmark and Portugal

Luis Teles de Carvalho, Ricardo; Jensen, Ole Michael; Tarelho, Luis A. C.; Olesen, Helge Rørdam

Creative Commons License Other

Publication date:

2015

Document Version

Publisher's PDF, also known as Version of record Link to publication from Aalborg University

Citation for published version (APA):

Luis Teles de Carvalho, R., Jensen, O. M., Tarelho, L. A. C., & Olesen, H. R. (2015). Particulate emissions from residential wood combustion: Improving estimations in Denmark and Portugal. Abstract from 11th International Conference on Carbonaceous Particles in the Atmosphere, Berkeley, United States.

http://iccpa.lbl.gov/presentations/carvalho-oral.pdf

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(2)

PARTICULATE EMISSIONS FROM RESIDENTIAL WOOD COMBUSTION:

IMPROVING ESTIMATIONS IN DENMARK AND PORTUGAL

INTERNATIONAL CONFERENCE ON CARBONACEOUS PARTICLES BERKELEY, USA

Ricardo L. Carvalho, Ole M. Jensen, Luís A. Tarelho, Helge R. Olesen

Danish Building Research Institute, Aalborg University, Denmark Centre for Environmental and Marine Studies, Aveiro University, Portugal Danish Centre for Environment and Energy, Aarhus University, Denmark

rlc@sbi.aau.dk

(3)

European Commission, Working Document on Possible Ecodesign and Energy Labelling Requirements for Local Space Heaters (2013) United Nations, Department of Economic and Social Affairs, Population Division (2013)

World Health Organization, Household Energy Database (2010)

Over 240 million people is relying on heating fireplaces and inefficient WBSs and boilers in the cold season

• Household heating is a major cause of permature deaths in Europe, North America and China

Fireplaces and wood-burning

stoves (WBSs) in more than 20% of the European households

• Secondary heating systems in areas with developed district heating grids

How to improve PM emission estimations from RWC in Europe?

Climate change threat

Global health risk

Global health risk

RWC ~

(4)

Secondary energy for cozyness (low wattage and mechanical vent.) Primary energy supply for heat

(high wattage and natural vent.)

High fuel loads & low tighness

Low fuel loads

& high tightness

HOUSEHOLD HEATING AND PM EMISSIONS IN WESTERN EUROPE (two case studies and new methods in the EU28)

Denmark

5,6 Mo

(12% rural)

42.916 km2

Portugal

10,4 Mo

(40% rural)

92.212 km2

43% of people

(<10% rural)

32% of area (of California)

= +

750.000 units 1.5 Mo

units

42%

25%

RWC units per dwelling

Well developed heating grid So, part of culture…

20-50% of wood heat Local resilience…

Up to 100% of wood heat

Heating typical

a single family house with NG

Costs 10% more In 2015 than in 2008 (ERSE, 2015)

(5)

OLD TRADITIONAL WBSs

Closed stove in Spain Carvalho, 2015 Fireplace in Europe

Open fire, 2014

(6)

NEW & NEW MODERN WBS

Swan labelled stove (NEW MODERN, after 2008) in Denmark Carvalho, 2014 Wood stove (NEW, before 2008) in Portugal

Carvalho, 2014

(7)

BOILERS AND COOKERS

Wood cooking boiler in Portugal Lareiras Pacinha , 2015 Residential wood boiler in Denmark

Perthshire biofuels, 2015

(8)

RWC in Denmark/Nordic region

~770,850 installations

26%

41%

30%

3%

Old closed New closed Modern

Boilers and cookers

uncertain…

T1: Lab to field studies, 2014

~1.6Mo users

per ~3.0Mo dwellings

[12] Incentive and Forced Technology. Danish Ministry of Environment. Virkemiddelkatalog for NOX, PM2.5, NMVOC og NH3, Miljøprojekt nr. 1514, 2013.

73%

27%

Non-users Users

[13] Forced Technology. Brændeforbrug i Danmark 2013.

21.920 TJ

(9)

RWC in Portugal/Mediterran region

~1.2Mo installations

43%

19%

20%

0% 18%

Fireplace Old closed New closed Modern

Boilers and cookers

~3.6 Mo users

Over ~3.4Mo dwellings

[1] C. Gonçalves, C. Alves, C. Pio. Inventory of fine particulate organic compound emissions from residential wood combustion in Portugal.

Atmospheric Environment, 50, 297-306, 2012.

66%

34%

Non-users Users

[14] Instituto Nacional de Estatística. Housing units of usual residence (No.) by Geographic localization (at the date of Census 2001) and Sewal disposal system; Decennialin Portugal, 2001.

T2: Field to lab.

studies, 2015

35.342 TJ +60% than DK!

(10)

AVAILABLE EMISSION INVENTORIES AND GAPS (PHONE SURVEYS)

[2] O. K. Nielsen, M. S. Plejdrup, M. Winther, M. H. Mikkelsen, M. Nielsen, S. Gyldenkærne, P. Fauser, R. Albrektsen, K. Hjelgaard, H. G. Bruun, M.

Thomsen. Annual Danish Annual Inventory report to UNECE, 2015.

[1] C. Gonçalves, C. Alves, C. Pio. Inventory of fine particulate organic compound emissions from residential wood combustion in Portugal.

Atmospheric Environment, 50, 297-306, 2012.

• Survey (2015) for ONLY 2133 people and 4 types of stoves…

• Average Efs on condensed particles with a controlled pressure chimney draft (Norwegian method)

• Spatial distribution from housing registration system (BBR)

• Survey (2012) for ONLY 2400 people and 2 types of systems…

• Standard Efs on condensed particles but with uncontrolled pressure chimeny draft

(prEN4711)

• Spatial distribution from one single study [1]

Denmark Portugal

𝐸 𝑃𝑀 = 𝑊𝑐 ∙ EFs

𝑛

𝑖=0

(11)

DANISH VS. PORTUGUESE PM2.5 EMISSION FACTORS?

(FIREPLACES, WOOD-LOG AND PELLET STOVES)

[12] Incentive, Forced Technology. Danish Ministry of Environment.

Virkemiddelkatalog for NOX, PM2.5, NMVOC og NH3, Miljøprojekt nr. 1514, 2013.

[1] C. Gonçalves, C. Alves, C. Pio. Inventory of fine particulate organic compound emissions from residential wood combustion in Portugal.

Atmospheric Environment, 50, 297-306, 2012.

[18] EMEP, 2013

T1: Lab to field studies, 2015 𝐸

𝑃𝑀

= 𝑊𝑐𝑖 ∙

𝑛

𝑖=0

EFsi T2: Lab to field

studies, 2014

0 200 400 600 800 1000 1200 1400 1600

fireplace old new modern new modern

gPM2. 5 /G J

Portugal Denmark

Used in the inventory

(12)

MAIN GAPS ON OFFICIAL EMISSION FACTORS?

[2] O. K. Nielsen, M. S. Plejdrup, M. Winther, M. H. Mikkelsen, M. Nielsen, S.

Gyldenkærne, P. Fauser, R. Albrektsen, K. Hjelgaard, H. G. Bruun, M.

Thomsen. Annual Danish Annual Inventory report to UNECE, 2015.

[1] C. Gonçalves, C. Alves, C. Pio. Inventory of fine particulate organic compound emissions from residential wood combustion in Portugal.

Atmospheric Environment, 50, 297-306, 2012.

• Approaches to mainstream emissions, not representing:

– Uncontrolled stove venting and household ventilation

(underpressure in real world)?

• Lab tests under ideal conditions do not represent situations where:

– Uncontrolled stove venting and household ventilation (under or over pressure in real world)?

Denmark Portugal

𝐸 𝑃𝑀 = 𝑊𝑐 ∙ EFs

𝑛

𝑖=0

Wet wood used in real-life NOT CONSIDERED…

Typical fuel loads vary from mean values…

(13)

RECALCULATIONS OF ANNUAL PM2.5 EMISSIONS?

[2] O. K. Nielsen, M. S. Plejdrup, M. Winther, M. H. Mikkelsen, M. Nielsen, S. Gyldenkærne, P. Fauser, R. Albrektsen, K. Hjelgaard, H. G. Bruun, M.

Thomsen. Annual Danish Annual Inventory report to UNECE, 2015.

[1] C. Gonçalves, C. Alves, C. Pio. Inventory of fine particulate organic compound emissions from residential wood combustion in Portugal.

Atmospheric Environment, 50, 297-306, 2012.

𝑬 𝑷𝑴 = 𝑊𝑐 ∙ EFs

𝑛

𝑖=0

0 5 10 15 20 25

wood consumption old

(TJ)

wood consumption

new (TJ)

PM2.5 emissions (kton)

Denmark Portugal PM2.5 emissions kton PM2.5

???

year-1

kg PM2.5 per capita

kton PM2.5

year-1 Share

Countries RWC RWC All sources %

Denmark 17,3? 3,1? 28,3 61%?

Portugal 11,0? 1,1 36,3 30%?

Underestimated emissions for Portuguese fireplaces?

Overestimated emissions

for new Danish stoves?

(14)

SPATIAL DISTRIBUTION OF PM2.5 EMISSIONS PER CASE

[15] Plejdrup, M.S., Nielsen, O-K. & Brandt, J., 2015: Development of a model for high resolution spatial distribution of emissions from residential wood combustion in Denmark. In prep.

.

[1] C. Gonçalves, C. Alves, C. Pio. Inventory of fine particulate organic compound emissions from residential wood combustion in Portugal.

Atmospheric Environment, 50, 297-306, 2012.

Portugal 𝑬 𝑷𝑴 = 𝑊𝑐 ∙ EFs

𝑛

𝑖=0

T1: Lab to field studies, 2014

T2: Field to lab.

studies, 2015

(15)

T1a. A PIONEER LAB-TO-FIELD TEST ON EF S IN DANISH DWELLINGS (by Glausius et al., DCE, Aarhus University, 2005)

[7] Glausius et al. 2005 (real-life measurements in 13 houses in Denmark)

990 g/GJ official Ef for old stoves

(2005/07)

[16] J. Illerup, T. Henriksen, T. Brændeovne og små kedler partikelemissioner og reduktionstiltag, 2007 (official laboratory tests)

[7] Glausius et al. 2005

(real-life measurements in 13 houses in Denmark)

Users behaviours can be the main reason

of variations on the PM 2.5 Efs!

(16)

T1b: LAB-TO-FIELD AIR QUALITY STUDY IN A DANISH VILLAGE (WOODUSE, DCE, Aarhus University, 2006/12)

WOODUSE: Slagslunde: 400 houses, 201 with wood stoves or boilers

[4] H.R. Olesen, P. Wåhlin, J. Illerup et al. Characteristics of residential wood combustion – results from a Danish case study, 2012 (experiments carried out in 2006/07)

(17)

TEOM_PM2.5

0 5 10 15 20 25

18-12- 2006 25-12- 2006 01-01- 2007 08-01- 2007 15-01- 2007 22-01- 2007 29-01- 2007 05-02- 2007 12-02- 2007 19-02- 2007 26-02- 2007

TEOM_PM2.5 (µgm

-3

)

Residential

Background

T1b: TEOM measured [PM 2.5 ] increment due to wood combustion during the 6-weeks period

[4] H.R. Olesen, P. Wåhlin, J. Illerup et al. Characteristics of residential wood combustion – results from a Danish case study, 2012

(experiments carried out in 2006/07)

TEOM (tapered element oscilating microbalance) is a continuous measurement method of atmospheric particles

(18)

T1: WOODUSE computated increment due to wood combustion for an average for 6-week period

Average at the monitor:

Measured: 1.97 µg/m3 Modelled (OML): 4.2 µg/m3

[4] H.R. Olesen, P. Wåhlin, J. Illerup et al. Characteristics of residential wood combustion – results from a Danish case study, 2012

(experiments carried out in 2006/07) OML is an atmospheric dispersion model

935 g/GJ (lab determ.) avEf Slangslunde used in the model

(2006/07)

𝑐𝑜𝑟𝑟𝑒𝑐𝑡𝑖𝑜𝑛 𝑓𝑎𝑐𝑡𝑜𝑟 = 𝑚𝑒𝑎𝑠𝑢𝑟𝑒𝑑 𝑎𝑣

𝑚𝑜𝑑𝑒𝑙𝑙𝑒𝑑 𝑎𝑣 = 1.97 𝑎𝑣

4.2 𝑎𝑣 = 0.47

(19)

T1b WOODUSE: LAB-TO-FIELD AIR QUALITY STUDY IN A DANISH VILLAGE (DCE, , Aarhus University, 2007/12)

𝑐𝑜𝑟𝑟. 𝑎𝑣. 𝐸𝐹 = 𝟎. 𝟒𝟕 ∙ 𝟗𝟑𝟓~𝟒𝟒𝟎 𝒈𝑷𝑴/𝑮𝑱

[4] H.R. Olesen, P. Wåhlin, J. Illerup et al. Characteristics of residential wood combustion – results from a Danish case study, 2012 (experiments carried out in 2006/07)

(20)

Dilution tunnel and dust-track Testing convection installation

[5] E.D. Vicente, M.A. Duarte, A.I. Calvo, T.F. Nunes, L. Tarelho, C.A. Alves. Emission of carbon monoxide, total hydrocarbons and particulate matter during wood combustion in a stove operating under distinct conditions, 2015.

T2: FIELD-TO-LAB IN PORTUGAL: performance test installation

(CESAM, Aveiro University, 2015)

(21)

[5] E.D. Vicente, M.A. Duarte, A.I. Calvo, T.F. Nunes, L. Tarelho, C.A. Alves. Emission of carbon monoxide, total hydrocarbons and particulate matter during wood combustion in a stove operating under distinct conditions, 2015.

T2: A NEW FIELD-TO-LAB APPROACH FOR AN IBERIAN WBSs (CESAM, Aveiro University, 2015)

For the dry softwood Pinus Pinaster (wood type on RWC in Portugal):

• Variations on fuel load may increase particulate emissions by more than 3 times comparing to official

emission factors used in previous inventories ”5.2±4.3 g/kgF”

• These variations might be even larger if we consider a common bottom ignition during lightning!

For the dry hardwood Fagus Sylvatica (typical fuel in Spain):

• Such operating practices did not change sigficantly…

-25%?

Technology controls..?

Official EF for

stoves (2012)

(22)

IAQ TEST: indoor [PM 2.5 ] during one week in the Autum when testing a wood stove (CESAM, Aveiro University, 2014)

0 0,5 1 1,5 2 2,5

08:24:00 10:48:00 13:12:00 15:36:00 18:00:00 20:24:00

Indoor PM2.5 concentration (mg/m3)

dia 1 dia 2 dia 3 dia 4 dia 5 dia 6 dia 7 dia 8

Indoor particules increase due to underpressure:

• Transport of particules from outdoors to indoors

• Indoor emissions when lightning (insuficcient draft)…

Lightning day 2 Lightning

test day 6 Lightning

test day 2

[17] Carvalho, R. L. Impactos de fogões a biomassa domésticos na qualidade do ar interior, estágio da Ordem dos Engenheiros, 2015.

(23)

• T h e c u r r e n t e s t i m a t i o n s a r e r a t h e r u n c e r t a i n d u e t o :

• F e w a v a i l a b l e s u r v e y s w i t h f e w r e s p o n d e n t s …

L i t t l e k n o w l e d g e o f r e p r e s e n t a t i v e E f s

• L i m i t e d k n o w l e d g e o n t h e s p a t i a l d i s t r i b u t i o n …

Conclusions and recommendations

• Improve activity data in conjunction with national chimney sweepers associations

• New testing methods and studies to determine real emissions, especially for old types of appliances (larger uncertainties) by:

Bringing the lab to field (quite expensive…)

Bringing the field to lab (economic, deep investigation on burning practices)

Modelling real-life household savings and mitigation effects

(24)

PARTICULATE EMISSIONS FROM RESIDENTIAL WOOD COMBUSTION:

IMPROVING ESTIMATIONS IN DENMARK AND PORTUGAL

INTERNATIONAL CONFERENCE ON CARBONACEOUS PARTICLES BERKELEY, USA

Ricardo L. Carvalho, Ole M. Jensen, Luís A. Tarelho, Helge R. Olesen

Danish Building Research Institute, Aalborg University, Denmark Centre for Environmental and Marine Studies, Aveiro University, Portugal Danish Centre for Environment and Energy, Aarhus University, Denmark

rlc@sbi.aau.dk

(25)

WBS use in Denmark and Portugal

Denmark Portugal

27%

42%

31% Old closed

New closed

Modern 53%

23%

24%

Fireplace Old closed New closed

21.920 TJ 35.342 TJ

[2] O. K. Nielsen, M. S. Plejdrup, M. Winther, M. H. Mikkelsen, M. Nielsen, S. Gyldenkærne, P. Fauser, R. Albrektsen, K. Hjelgaard, H. G. Bruun, M.

Thomsen. Annual Danish Annual Inventory report to UNECE, 2015.

[1] C. Gonçalves, C. Alves, C. Pio. Inventory of fine particulate organic compound emissions from residential wood combustion in Portugal.

Atmospheric Environment, 50, 297-306, 2012.

(26)

SURVEYS (2012/13): REAL WOOD CONSUMPTION AND TRANSITIONS (T)?

[2] O. K. Nielsen, M. S. Plejdrup, M. Winther, M. H. Mikkelsen, M. Nielsen, S. Gyldenkærne, P. Fauser, R. Albrektsen, K. Hjelgaard, H. G. Bruun, M.

Thomsen. Annual Danish Annual Inventory report to UNECE, 2015.

[1] C. Gonçalves, C. Alves, C. Pio. Inventory of fine particulate organic compound emissions from residential wood combustion in Portugal.

Atmospheric Environment, 50, 297-306, 2012.

RWC Activity data Respondents Dwellings

Per pop. Stoves Share Users or Per cap.

Old stoves (before2008)

New stoves

(after 2008) WBSs Boilers and

cookers Ref.

Countries All All All All All Users Fireplace Old closed New

closed Modern All All All

Denmark 2013

Number (Mo)

2.133 x10-3

(3,0/10,4)

x106 0,8x106 27% 1,5x106 - 202.500 315.000 232.500 750.000 20.845

[9] Forced tech, 2013 [2] Nielsen, 2015 Wood

consump.

(TJ y-1)

- - 21.920 3.9 - 4.087 8.622 5.936 18.645 3.275

Portugal 2012

Number

(Mo) 2.387 (3,4/5,6)

x106 1.5x106 34% 3,6x106 645.818 282.903 294.333 - 1.161.221 272.901 [1] Goncalves, 2012 [10] INE, 2011 Wood

consump.

(TJ y-1)

- -

35.342 3.6 17.184 6.512 7.410 - 31.105 4.237

𝐸

𝑃𝑀

= 𝑾𝒄𝑖 ∙

𝑛 𝑖=0

EFsi T1: Lab to field

studies, 2014

T2: field to lab

studies, 2015

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